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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Discussion papers | Copyright
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 05 Nov 2018

Research article | 05 Nov 2018

Review status
This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Measurement Techniques (AMT).

An instrument for the rapid quantification of PM oxidative potential: the Particle Into Nitroxide Quencher (PINQ)

Reece Alexander Brown1, Svetlana Stevanovic1,3, Steven Bottle2, and Zoran Ristovski1,2 Reece Alexander Brown et al.
  • 1ILAQH (International Laboratory of Air Quality and Health), Queensland University of Technology, 2 George St, Brisbane, 4000 QLD, Australia
  • 2School of Chemistry, Physics and Mechanical Engineering, Queensland University of Technology (QUT), Brisbane, 4000 QLD, Australia
  • 3School of Engineering, Deakin University, VIC 3216, Australia

Abstract. Presence or generation of reactive oxygen species (ROS) on/by particulate matter (PM) have been implicated in PM-induced health effects. Methodologies to quantify ROS concentrations vary widely both in detection and collection methods. However, there is currently an increasing emphasis on rapid collection and measurement due to observations of short half-live ROS. To address this problem, this manuscript details the design and characterization of a novel instrument named the Particle Into Nitroxide Quencher (PINQ). This instrument combines the BPEAnit ROS assay in conjunction with a purpose-built aerosol collection device, the insoluble aerosol collector (IAC). The IAC continuously collects PM regardless of size or chemistry directly into a liquid sample with a collection efficiency of 0.98 and a low cut-off size of < 20 nm. The sampling time resolution of the PINQ is one minute, with a limit of detection (LOD) of 0.08 nmol m−3 in equivalent BPEAnit-Me concentration per volume of air. This high sample time resolution and sensitivity is achieved due a combination of the highly concentrated IAC liquid sample and the rapid reaction and stability of the BPEAnit probe.

Reece Alexander Brown et al.
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Status: open (until 31 Dec 2018)
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Reece Alexander Brown et al.
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