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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union

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https://doi.org/10.5194/amt-2017-282
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
Research article
04 Aug 2017
Review status
This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Measurement Techniques (AMT).
A new non-resonant laser-induced fluorescence instrument for the airborne in situ measurement of formaldehyde
Jason M. St. Clair1,2, Andrew K. Swanson1,3, Steven A. Bailey1, Glenn M. Wolfe1,2, Josette E. Marrero4, Laura T. Iraci4, John G. Hagopian5,6, and Thomas F. Hanisco1 1Atmospheric Chemistry and Dynamics Laboratory, NASA Goddard Space Flight Center, Greenbelt, MD, 20771, USA
2Joint Center for Earth Systems Technology, University of Maryland Baltimore County, Baltimore, MD, 21228, USA
3Goddard Earth Sciences Technology and Research, Universities Space Research Association, Columbia, MD, 21046, USA
4Atmospheric Science Branch, NASA Ames Research Center, Moffett Field, CA, 94035, USA
5Lambda Consulting/Advanced Nanophotonics, Harwood, MD, 20776, USA
6Optics Branch, Instrument Systems and Technology Division, NASA Goddard Space Flight Center, Greenbelt, MD, 20771, USA
Abstract. A new in situ instrument for gas-phase formaldehyde (HCHO), COmpact Formaldehyde FluorescencE Experiment (COFFEE), is presented. COFFEE utilizes non-resonant laser-induced fluorescence (NR-LIF) to measure HCHO, with 300 mW of 40 kHz 355 nm laser output exciting multiple HCHO absorption features. The resulting HCHO fluorescence is collected at 5 ns resolution, and the fluorescence time profile is fit to yield the ambient HCHO mixing ratio. Typical 1-σ precision at ~ 0 pptv HCHO is 150 pptv for 1 s data. The compact instrument was designed to operate with minimal in-flight operator interaction and infrequent maintenance (1–2 times per year). COFFEE fits in the wing pod of the Alpha Jet stationed at NASA Ames Research Center and has successfully collected HCHO data on 27 flights through 2017 March. The frequent flights, combined with a potentially long-term data set, makes the Alpha Jet a promising platform for validation of satellite-based column HCHO.

Citation: St. Clair, J. M., Swanson, A. K., Bailey, S. A., Wolfe, G. M., Marrero, J. E., Iraci, L. T., Hagopian, J. G., and Hanisco, T. F.: A new non-resonant laser-induced fluorescence instrument for the airborne in situ measurement of formaldehyde, Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-282, in review, 2017.
Jason M. St. Clair et al.
Jason M. St. Clair et al.
Jason M. St. Clair et al.

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Short summary
Formaldehyde is an abundant, photochemically influential trace species in the Earth’s atmosphere. We present a new instrument for measuring atmospheric formaldehyde using a laser-based measurement technique that is more compact and lower cost than previous laser-based formaldehyde instruments. The instrument is part of the Alpha Jet Atmospheric eXperiment (AJAX) payload at NASA Ames Research Center and has collected data on 27 flights between December 2015 and March 2017.
Formaldehyde is an abundant, photochemically influential trace species in the Earth’s...
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