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<article language="en">
	<journal>
		<journal_title>Atmospheric Measurement Techniques Discussions</journal_title>
		<journal_url>www.atmos-meas-tech-discuss.net</journal_url>
		<eissn>1867-8610</eissn>
		<volume_number>2</volume_number>
		<issue_number>6</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/amtd-2-2851-2009</doi>
	<article_url>http://www.atmos-meas-tech-discuss.net/2/2851/2009/</article_url>
	<abstract_html>http://www.atmos-meas-tech-discuss.net/2/2851/2009/amtd-2-2851-2009.html</abstract_html>
	<fulltext_pdf>http://www.atmos-meas-tech-discuss.net/2/2851/2009/amtd-2-2851-2009.pdf</fulltext_pdf>
	<start_page>2851</start_page>
	<end_page>2880</end_page>
	<publication_date>2009-11-02</publication_date>
	<article_title content_type="html">Mobile MAX-DOAS observations of tropospheric trace gases</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>T. Wagner</name>
			<email>thomas.wagner@mpch-mainz.mpg.de</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>O. Ibrahim</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>R. Shaiganfar</name>
		</author>
		<author numeration="4" affiliations="2">
			<name>U. Platt</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Max-Planck-Institute for Chemistry, Mainz, Germany</affiliation>
		<affiliation numeration="2" content_type="html">Institute for Environmental Physics, University of Heidelberg, Germany</affiliation>
	</affiliations>
	<abstract content_type="html">From Multi-Axis- (MAX-) DOAS observations information on tropospheric trace gases close to
      the surface and up to the free troposphere can be obtained. Usually MAX-DOAS observations
      are performed at fixed locations, which allows to retrieve the diurnal variation of
      tropospheric species at that location. Alternatively, MAX-DOAS observations can also be made
      on mobile platforms like cars, ships or aircrafts. Then, in addition to the vertical (and
      temporal) distribution, also the horizontal variation of tropospheric trace gases can be
      measured. Such information is important for the quantitative comparison with model
      simulations, study of transport processes, and for the validation of tropospheric trace gas
      products from satellite observations. However, for MAX-DOAS observations from mobile
      platforms, the standard analysis techniques for MAX-DOAS observations can usually not be
      applied, because the probed airmasses can change rapidly between successive measurements. In
      this study we introduce a new technique which overcomes these problems and allows the
      exploitation of the full information content of mobile MAX-DOAS observations. Our method can
      also be applied to MAX-DOAS observations made at fixed locations in order to improve the
      accuracy especially in cases of strong winds. We apply the new technique to MAX-DOAS
      observations made during an automobile trip from Brussels to Heidelberg.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Brinksma, E J., Pinardi, G., Braak, R., Volten, H., Richter, A., Schönhardt, A., van Roozendael, M., Fayt, C., Hermans, C., Dirksen, R J., Vlemmix, T., Berkhout, A J C., Swart, D P J., Ötjen, H., Wittrock, F., Wagner, T., Ibrahim, O W., de Leeuw, G., Moerman, M., Curier, R L., Celarier, E A., Knap, W H., Veefkind, J P., Eskes, H J., Allaart, M., Rothe, R., Piters, A J M., and Levelt,~P F.: The 2005 and 2006 DANDELIONS \chemNO_2 and Aerosol Validation Campaigns, J. Geophys. Res., 113, D16S46, doi:10.1029/2007JD008808, 2008. </reference>
		<reference numeration="2" content_type="text"> Bogumil, K., Orphal, J., Homann, T., Voigt, S., Spietz, P., Fleischmann, O C., Vogel, A., Hartmann, M., Bovensmann, H., Frerik, J., and Burrows, J P.: Measurements of molecular absorption spectra with the SCIAMACHY pre-flight model: instrument characterization and reference data for atmospheric remote-sensing in the 230–2380 \unitnm region, J. Photochem. Photobiol. A., 157, 167–184, 2003. </reference>
		<reference numeration="3" content_type="text"> Bovensmann, H., Burrows, J P., Buchwitz, M., Frerick, J., No\&quot;el, S., Rozanov, V V., Chance, K V., and Goede, A H P.: SCIAMACHY – mission objectives and measurement modes, J. Atmos. Sci., 56(2), 127–150, 1999. </reference>
		<reference numeration="4" content_type="text"> Bruns, M., Buehler, S A., Burrows, J P., Richter, A., Rozanov, A., Wang, P., Heue, K P., Platt, U., Pundt, I., and Wagner, T.: \chemNO_2 Profile retrieval using airborne multi axis UV-visible skylight absorption measurements over central Europe, Atmos. Chem. Phys., 6, 3049–3058, 2006. </reference>
		<reference numeration="5" content_type="text"> Celarier, E A., Brinksma, E J., Gleason, J F., Veefkind, J P., Cede, A., Herman, J R., Ionov, D., Goutail, F., Pommereau, J-P., Lambert, J-C., van Roosendael, M., Pinardi, G., Richter, A., Wagner, T., Bojkov, B., Mount,~G., Spinei,~E., Chen,~C M., Pongetti,~T J., Sander,~S P., Bucsela,~E J., Wenig, M O., Swart,~D P J., Volten,~H., Kroon,~M., and Levelt, P F.: Validation of ozone monitoring instrument nitrogen dioxide columns, J. Geophys. Res., 113, D15S15, doi:10.1029/2007JD008908, 2008. </reference>
		<reference numeration="6" content_type="text"> Dix, B., Brenninkmeijer, C A M., Frieß, U., Wagner, T., and Platt, U.: Airborne multi-axis DOAS measurements of atmospheric trace gases on CARIBIC long-distance flights, Atmos. Meas. Tech. Discuss., 2, 265–301, 2009. </reference>
		<reference numeration="7" content_type="text"> Fayt, C. and van Roozendael, M.: WinDOAS 2.1 Software User Manual, (http://www.oma.be/GOME/GOMEBrO/WinDOAS-SUM-210b.pdf), 2001. </reference>
		<reference numeration="8" content_type="text"> Fietkau, S., Medeke, T., Richter, A., Sheode, N., Sinnhuber, B.-M., Wittrock, F., Theys, N., van Roozendael, M., and Burrows, J. P.: Ground-based measurements of tropospheric and stratospheric bromine monoxide above Nairobi (1&amp;deg; S, 36&amp;deg; E), Atmos. Chem. Phys. Discuss., 7, 6527–6555, 2007. </reference>
		<reference numeration="9" content_type="text"> Frieß, U., Monks, P S., Remedios, J J., Rozanov, A., Sinreich, R., Wagner, T., and Platt, U.: MAX-DOAS \chemO_4 measurements: A~new technique to derive information on atmospheric aerosols. (II) Modelling studies, J. Geophys. Res., 111, D14203, doi:10.1029/2005JD006618, 2006. </reference>
		<reference numeration="10" content_type="text"> Grainger, J F. and Ring, J.: Anomalous Fraunhofer line profiles, Nature, 193, p 762, 1962. </reference>
		<reference numeration="11" content_type="text"> Greenblatt, G D., Orlando, J J., Burkholder, J B., and Ravishankara, A R.: Absorption measurements of oxygen between 330 and 1140 \unitnm, J. Geophys. Res., 95, 18577–18582, 1990. </reference>
		<reference numeration="12" content_type="text"> Heckel, A., Richter, A., Tarsu, T., Wittrock, F., Hak, C., Pundt, I., Junkermann, W., and Burrows, J P.: MAX-DOAS measurements of formaldehyde in the Po-Valley, Atmos. Chem. Phys., 5, 909–918, 2005. </reference>
		<reference numeration="13" content_type="text"> Heue, K.-P., Richter, A., Bruns, M., Burrows, J P., v. Friedeburg, C., Platt, U., Pundt, I., Wang, P., and Wagner, T.: Validation of SCIAMACHY tropospheric \chemNO_2-columns with AMAXDOAS measurements, Atmos. Chem. Phys., 5, 1039–1051, 2005. </reference>
		<reference numeration="14" content_type="text"> Hönninger, G. and Platt, U.: Observations of \chemBrO and its vertical distribution during surface ozone depletion at Alert, Atmos. Environ., 36, 2481–2490, 2002. </reference>
		<reference numeration="15" content_type="text"> Hönninger, G., von Friedeburg, C., and Platt, U.: Multi axis differential optical absorption spectroscopy (MAX-DOAS), Atmos. Chem. Phys., 4, 231–254, 2004. </reference>
		<reference numeration="16" content_type="text"> Hönninger, G., Leser, H., Sebastian, O., and Platt, U.: Ground-based measurements of halogen oxides at the Hudson Bay by active long path DOAS and passive MAX-DOAS, Geophys. Res. Lett. 31, L04111, doi:10.1029/2003GL018982, 2004b. </reference>
		<reference numeration="17" content_type="text"> Ibrahim, O.: Applications on Ground-based Tropospheric Measurements using Multi-Axis Differential Optical Absorption Spectroscopy, PhD-thesis, University of Heidelberg, Germany, 2009. </reference>
		<reference numeration="18" content_type="text"> Irie, H., Kanaya, Y., Akimoto, H., Tanimoto, H., Wang, Z., Gleason, J F., and Bucsela, E J.: Validation of OMI tropospheric \chemNO_2 column data using MAX-DOAS measurements deep inside the North China Plain in June 2006: Mount Tai Experiment 2006, Atmos. Chem. Phys., 8, 6577–6586, 2008. </reference>
		<reference numeration="19" content_type="text"> Johansson, M., Galle, B., Yu, T., Tang, L., Chen, D., Li, H., Li, J X., and Zhang, Y.: Quantification 20 of total emission of air pollutants from Beijing using mobile mini-DOAS, Atmos. Environ., 42, 6926–6933, 2008. </reference>
		<reference numeration="20" content_type="text"> Johansson, M., Rivera, C., de Foy, B., Lei, W., Song, J., Zhang, Y., Galle, B., and Molina, L.: Mobile mini-DOAS measurement of the outflow of NO2 and HCHO from Mexico City, Atmos. Chem. Phys., 9, 5647–5653, 2009 </reference>
		<reference numeration="21" content_type="text"> Kraus, S.: DOASIS, A~Framework Design for DOAS, PhD-thesis, University of Mannheim (http://hci.iwr.uni-heidelberg.de/publications/dip/2006/Kraus_PhD2006.pdf), 2006. </reference>
		<reference numeration="22" content_type="text"> Kurucz, R L., Furenlid, I. Brault, J., and Testerman, L.: Solar flux atlas from 296 \unitnm to 1300 \unitnm, National Solar Observatory Atlas, No 1, 1984. </reference>
		<reference numeration="23" content_type="text"> Leser, H., Hönninger, G., and Platt, U.: MAX-DOAS measurements of \chemBrO and \chemNO_2 in the marine boundary layer, Geophys. Res. Lett., 30(10), 1537, doi:10.1029/2002GL015811, 2003. </reference>
		<reference numeration="24" content_type="text"> Levelt, P F. and Noordhoek, R.: OMI Algorithm Theoretical Basis Document Volume I: OMI Instrument, Level 0-1b Processor, Calibration &amp; Operations, Tech. Rep. ATBD-OMI-01, Version 1.1, August 2002. </reference>
		<reference numeration="25" content_type="text"> Marquard, L C., Wagner, T., and Platt, U.: Improved air mass factor concepts for scattered radiation differential optical absorption spectroscopy of atmospheric species, J. Geophys. Res.,105, 1315–1327, 2000. </reference>
		<reference numeration="26" content_type="text"> Noxon, J F., Whipple, E C., and Hyde, R S.: Stratospheric \chemNO_2, 1 Observational method and behaviour at midlatitudes, J. Geophys. Res., 84, 5047–5076, 1979. </reference>
		<reference numeration="27" content_type="text"> Perliski, L M. and Solomon, S.: On the evaluation of air mass factors for atmospheric near-ultraviolet and visible absorption spectroscopy, J. Geophys. Res., 98, 10363–10374, 1993. </reference>
		<reference numeration="28" content_type="text"> Platt, U. and Stutz, J.: Differential Optical Absorption Spectroscopy, Principles and Applications, Springer, Berlin, 2008. </reference>
		<reference numeration="29" content_type="text"> Rothman, L S., Jacquemart, D., Barbe, A., Benner, D C., Birk, M., Brown, L R., Carleer, M R., Chackerian, C. Jr., Chance, K., Coudert, L H., Dana, V., Devi, V M., Flaud, J.-M., Gamache, R R., Goldman, A., Hartmann, J.-M., Jucks, K W., Maki, A G., Mandin, J.-Y., Massie, S T., Orphal, J., Perrin, A., Rinsland, C P., Smith, M A H., Tennyson, J., Tolchenov, R N., Toth, R A., Vander Auwera, J., Varanasi, P., and Wagner G.: The HITRAN 2004 molecular spectroscopic database, J. Quant. Spectrosc. Ra., 96 139–204, 2005. </reference>
		<reference numeration="30" content_type="text"> Sinreich, R., Frieß, U., Wagner, T., and Platt, U.: Multi axis differential optical absorption spectroscopy (MAX-DOAS) of gas and aerosol distributions, Faraday Discuss., 130, 153, doi:10.1039/b419274, 2005. </reference>
		<reference numeration="31" content_type="text"> Solomon, S., Schmeltekopf, A L., and Sanders, R W.: On the interpretation of zenith sky absorption measurements, J. Geophys. Res., 92, 8311–8319, 1987. </reference>
		<reference numeration="32" content_type="text"> Stutz, J. and Platt, U.: Numerical analyses and estimation of the statistical error of differential optical absorption spectroscopy measurements with least square methods, Appl. Opt., 35, 6041–6053, 1996. </reference>
		<reference numeration="33" content_type="text"> Theys, N., Van Roozendael, M., Hendrick, F., Fayt, C., Hermans, C., Baray, J.-L., Goutail, F., Pommereau, J.-P., and De Mazière, M.: Retrieval of stratospheric and tropospheric \chemBrO columns from multi-axis DOAS measurements at Reunion Island (21\degree S, 56\degree E), Atmos. Chem. Phys., 7, 4733–4749, 2007. </reference>
		<reference numeration="34" content_type="text"> Vandaele, A C., Hermans, C., Simon, P C., Carleer, M., Colin, R., Fally, S., Mérienne, M.-F., Jenouvrier, A., and Coquart, B.: Measurements of the \chemNO_2 Absorption Cross-section from 42 000 \unitcm^-1 to 10 000 \unitcm^-1 (238–1000 \unitnm) at 220 \unitK and 294 \unitK, J. Quant. Spectrosc. Radiat. Transfer, 59, 171–184, 1997. </reference>
		<reference numeration="35" content_type="text"> van Roozendael, M., Fayt, C., Post, P., Hermans, C., Lambert, J.-C.: Retrieval of \chemBrO and \chemNO_2 from UV-Visible Observations, in: Sounding the Troposphere From Space: A~New Era for Atmospheric Chemistry, edited by: Borrell, P., Borrell, P. M., Burrows, J. P., and Platt, U., Springer-Verlag, ISBN:3-540-40873-8, 2003. </reference>
		<reference numeration="36" content_type="text"> Volk, R.: Auto-MAX-DOAS, Diploma thesis, University of Heidelberg, 2008. </reference>
		<reference numeration="37" content_type="text"> Wagner, T., Dix, B., v. Friedeburg, C., Frieß, U., Sanghavi, S., Sinreich, R., and Platt, U.: MAX-DOAS \chemO_4 measurements – a~new technique to derive information on atmospheric aerosols. (I) Principles and information content, J. Geophys. Res., 109, D22205, doi:10.1029/2004JD004904, 2004. </reference>
		<reference numeration="38" content_type="text"> Wagner, T., Burrows, J. P., Deutschmann, T., Dix, B., von Friedeburg, C., Frieß, U., Hendrick, F., Heue, K.-P., Irie, H., Iwabuchi, H., Kanaya, Y., Keller, J., McLinden, C. A., Oetjen, H., Palazzi, E., Petritoli, A., Platt, U., Postylyakov, O., Pukite, J., Richter, A., van Roozendael, M., Rozanov, A., Rozanov, V., Sinreich, R., Sanghavi, S., and Wittrock, F.: Comparison of box-air-mass-factors and radiances for Multiple-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) geometries calculated from different UV/visible radiative transfer models, Atmos. Chem. Phys., 7, 1809–1833, 2007a. </reference>
		<reference numeration="39" content_type="text"> Wagner, T., Ibrahim, O., Sinreich, R., Frieß, U., von Glasow, R., and Platt, U.: Enhanced tropospheric \chemBrO over Antarctic sea ice in mid winter observed by MAX-DOAS on board the research vessel Polarstern, Atmos. Chem. Phys., 7, 3129–3142, 2007b. </reference>
		<reference numeration="40" content_type="text"> Wagner, T., Deutschmann, T., and Platt, U.: Determination of aerosol properties from MAX-DOAS observations of the Ring effect, Atmos. Meas. Tech., 2, 495–512, 2009. </reference>
		<reference numeration="41" content_type="text"> Wang, P., Richter, A., Bruns, M., Rozanov, V V., Burrows, J. P., Heue, K.-P., Wagner, T., Pundt, I., and Platt, U.: Measurements of tropospheric \chemNO_2 with an airborne multi-axis DOAS instrument, Atmos. Chem. Phys., 5, 337–343, 2005. </reference>
		<reference numeration="42" content_type="text"> Wang, P., Richter, A., Bruns, M., Burrows, J P., Scheele, R., Junkermann, W., Heue, K.-P., Wagner, T., Platt, U., and Pundt, I.: Airborne multi-axis DOAS measurements of tropospheric \chemSO_2 plumes in the Po-valley, Italy, Atmos. Chem. Phys., 6, 329–338, 2006.  </reference>
		<reference numeration="43" content_type="text"> Wittrock, F., Oetjen, H., Richter, A., Fietkau, S., Medeke, T., Rozanov, A., and Burrows, J. P.: MAX-DOAS measurements of atmospheric trace gases in Ny-Ålesund~– Radiative transfer studies and their application, Atmos. Chem. Phys., 4, 955–966, 2004. </reference>
	</references>
</article>

