<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-meas-tech-discuss.net/inc/amtd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Measurement Techniques Discussions</journal_title>
		<journal_url>www.atmos-meas-tech-discuss.net</journal_url>
		<eissn>1867-8610</eissn>
		<volume_number>1</volume_number>
		<issue_number>1</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/amtd-1-249-2008</doi>
	<article_url>http://www.atmos-meas-tech-discuss.net/1/249/2008/</article_url>
	<abstract_html>http://www.atmos-meas-tech-discuss.net/1/249/2008/amtd-1-249-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-meas-tech-discuss.net/1/249/2008/amtd-1-249-2008.pdf</fulltext_pdf>
	<start_page>249</start_page>
	<end_page>279</end_page>
	<publication_date>2008-11-27</publication_date>
	<article_title content_type="html">Six years of total ozone column measurements from SCIAMACHY nadir observations</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>C. Lerot</name>
			<email>christophe.lerot@aeronomie.be</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>M. Van Roozendael</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>J. van Geffen</name>
		</author>
		<author numeration="4" affiliations="1">
			<name>J. van Gent</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>C. Fayt</name>
		</author>
		<author numeration="6" affiliations="2">
			<name>R. Spurr</name>
		</author>
		<author numeration="7" affiliations="3">
			<name>G. Lichtenberg</name>
		</author>
		<author numeration="8" affiliations="3">
			<name>A. von Bargen</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, Belgium</affiliation>
		<affiliation numeration="2" content_type="html">RT Solutions, Inc., Cambridge, Massachusetts, USA</affiliation>
		<affiliation numeration="3" content_type="html">German Aerospace Center (DLR), P.O. Box 1116, 82234 Wessling, Germany</affiliation>
	</affiliations>
	<abstract content_type="html">Total O&lt;sub&gt;3&lt;/sub&gt; columns have been retrieved from six years of SCIAMACHY nadir UV
radiance measurements using SDOAS, an adaptation of the GDOAS algorithm
previously developed at BIRA-IASB for the GOME instrument. GDOAS and SDOAS
have been implemented by the German Aerospace Center (DLR) in the version 4
of the GOME Data Processor (GDP) and in version 3 of the SCIAMACHY Ground
Processor (SGP), respectively. The processors are being run at the DLR
processing centre on behalf of the European Space Agency (ESA). We first
focus on the description of the SDOAS algorithm with particular attention to
the impact of uncertainties on the reference O&lt;sub&gt;3&lt;/sub&gt; absorption cross-sections.
Second, the resulting SCIAMACHY total ozone data set is globally evaluated
through large-scale comparisons with results from GOME and OMI as well as
with ground-based correlative measurements. The various total ozone data sets
are found to agree within 2% on average. However, a negative trend of
0.2â€“0.4%/year has been identified in the SCIAMACHY O&lt;sub&gt;3&lt;/sub&gt; columns; this
probably originates from instrumental degradation effects that have not yet
been fully characterized.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Bass, A. M. and Paur, R. J.: The ultraviolet cross-sections of ozone, I, The measurements, in: Atmospheric Ozone, edited by: Zerefos, C. S., Ghazi, A., and Reidel, D., Norwell, Mass., 606â€“610, 1985. </reference>
		<reference numeration="2" content_type="text"> Bhartia, P. K.: OMI algorithm theoretical basis document, 2, OMI ozone products, NASA Goddard Space Flight Center, Greenbelt, Maryland, USA, available at: http://eospso.gsfc.nasa.gov/eos_homepage/for_scientists/atbd/viewInstrument.php?instrument=13, 2002. </reference>
		<reference numeration="3" content_type="text"> Bodeker, G. E. and Waugh, D. W. (Lead Authors), Akiyoshi, H., Braesicke, P., Eyring, V., Fahey, D. W., Manzini, E., Newchurch, M. J., Portmann, R. W., Robock, A., Shine, K. P., Steinbrecht, W., and Weatherhead, E. C.: The Ozone Layer in the 21st Century, Chapter 6 in Scientific Assessment of Ozone Depletion: 2006, Global Ozone Research and Monitoring Project-Report No 50, World Meteorological Organization, Geneva, Switzerland, 572 pp., 2007.  </reference>
		<reference numeration="4" content_type="text"> Boersma, K. F., Eskes, H. J., and Brinksma, E. J.: Error analysis for tropospheric NO&lt;sub&gt;2&lt;/sub&gt; retrieval from space, J. Geophys. Res., 109, D04311, doi:10.1029/2003JD003962, 2004. </reference>
		<reference numeration="5" content_type="text"> Bogumil, K., Orphal, J., Homann, T., Voigt, S., Spietz, P., Fleischmann, O. C., Vogel, A., Hartmann, M., Bovensmann, H., Frerick, J., and Burrows, J. P.: Measurements of molecular absorption spectra with the SCIAMACHY pre-flight model: instrument characterization and reference data for atmospheric remote-sensing in the 230â€“2380 nm region, J. Photochem. Photobiol. A., 157, 167â€“184, 2003. </reference>
		<reference numeration="6" content_type="text"> Bovensmann, H., Burrows, J., Buchwitz, M., Frerick, J., Noel, S., Rozanov, V., Chance, K., and Goede, A.: SCIAMACHY: Mission objectives and measurement modes, J. Atmos. Sci., 56, 127â€“150, 1999. </reference>
		<reference numeration="7" content_type="text"> Bramstedt, K.: Calculation of SCIAMACHY M-Factors, TN IFE-SCIA-TN-2007-01-CalcMFactor, Issue 1, Institute of Environmental Physics, Bremen, available at: http://www.iup.uni-bremen.de/sciamachy/mfactors/mfactor-TN-1-0.pdf, 2008. </reference>
		<reference numeration="8" content_type="text"> Brion, J., Chakir, A., Daumont, D., and Malicet, J.: High-resolution laboratory absorption cross sections of O&lt;sub&gt;3&lt;/sub&gt;. Temperature effect, Chem. Phys. Lett., 213(5â€“6), 610â€“612, 1993. </reference>
		<reference numeration="9" content_type="text"> Burrows, J. P., Weber, M., Buchwitz, M., Rozanov, V., LadstÃ¤tter-Weissenmayer, A., Richter, A., DeBeek, R., Hoogen, R., Bramstedt, K., Eichmann, K.-U., Eisinger, M., and Perner, D.: The Global Ozone Monitoring Experiment (GOME): mission concept and first scientific results, J. Atmos. Sci., 56, 151â€“175, 1999a. </reference>
		<reference numeration="10" content_type="text"> Burrows, J., Richter, A., Dehn, A., Deters, B., Himmelmann, S., Voigt, S., and Orphal, J.: Atmospheric remote sensing reference data from GOME: Part 2. Temperature-dependent absorption cross-sections of O&lt;sub&gt;3&lt;/sub&gt; in the 231â€“794 nm range, J. Quant. Spectrosc. Radiat. Transfer, 61, 509â€“517, 1999b. </reference>
		<reference numeration="11" content_type="text"> Chance, K. and Spurr, R.: Ring effect studies: Rayleigh scattering including molecular parameters for rotational Raman scattering, and the Fraunhofer spectrum, Appl. Opt., 36, 5224â€“5230, 1997. </reference>
		<reference numeration="12" content_type="text"> Coldewey-Egbers, M., Weber, M., Lamsal, L. N., de Beek, R., Buchwitz, M., and Burrows, J. P.: Total ozone retrieval from GOME UV spectral data using the weighting function DOAS approach, Atmos. Chem. Phys., 5, 1015â€“1025, 2005. </reference>
		<reference numeration="13" content_type="text"> Daumont, M., Brion, J., Charbonnier, J., and Malicet, J.: Ozone UV spectroscopy, I: Absorption cross-sections at room temperature, J. Atmos. Chem., 15, 145â€“155, 1992. </reference>
		<reference numeration="14" content_type="text"> Eskes, H. J., van der A, R. J., Brinksma, E. J., Veefkind, J. P., de Haan, J. F., and Valks, P. J. M.: Retrieval and validation of ozone columns derived from measurements of SCIAMACHY on Envisat, Atmos. Chem. Phys. Discuss., 5, 4429-4475, 2005. </reference>
		<reference numeration="15" content_type="text"> Frerick, J. and von Bargen, A.: SCIAMACHY Level 1b-1c Processing - The SciaL1c Command-line Tool Software User&apos;s Manual, ENV-SUM-DLR-SCIA-0071, Issue 6.0/B, available at: http://earth.esa.int/services/SciaL1C_tool/SciaL1c_SUM_6.0B.pdf, 2007. </reference>
		<reference numeration="16" content_type="text"> Herman, J. R. and Celarier, E. A.: Earth surface reflectivity climatology at 340â€“380 nm from TOMS data, J. Geophys. Res., 102(D23), 28 003â€“28 012, doi:10.1029/97JD02074, 1997. </reference>
		<reference numeration="17" content_type="text"> Koelemeijer, R. B. A., Stammes, P., Hovenier, J. W., and de Haan, J. F.: A fast method for retrieval of cloud parameters using oxygen A band measurements from the Global Ozone Monitoring Experiment, J. Geophys. Res., 106(D4), 3475â€“3490, 2001. </reference>
		<reference numeration="18" content_type="text"> Koelemeijer, R. B. A., de Haan, J. F., Hovenier, J. W., and Stammes, P.: A database of spectral surface reflectivity in the range 335â€“772 nm derived from 5.5 years of GOME observations, J. Geophys. Res., 108(D2), 4070, doi:10.1029/2002JD002429, 2003. </reference>
		<reference numeration="19" content_type="text"> Kokhanovsky, A. A., Rozanov, V. V., Vountas, M., Lotz, W., Bovensmann, H., and Burrows, J. P.: SCIAMACHY 1b to 2 OL Processing, Algorithm Theoretical Basis Document, Semi-Analytical CloUd Retrieval Algorithm for SCIAMACHY/ENVISAT, ENV-ATB-IFE-SCIA-0003, Issue 2.0, available at: http://earth.esa.int/pub/ESA_DOC/ENVISAT/SCIAMACHY/ENVI95.pdf, 2008. </reference>
		<reference numeration="20" content_type="text"> Levelt, P. F., van den Oord, G. H. J., Dobber, M. R., Malkki, A., Visser, H., de Vries, J., Stammes, P., Lundell, J. O. V., and Saari, H.: The Ozone Monitoring Instrument, IEEE Trans. Geosc. Rem. Sens., 44(5), 1093â€“1101, 2006. </reference>
		<reference numeration="21" content_type="text"> Lichtenberg, G., Kleipool, Q., Krijger, J. M., van Soest, G., van Hees, R., Tilstra, L. G., Acarreta, J. R., Aben, I., Ahlers, B., Bovensmann, H., Chance, K., Gloudemans, A. M. S., Hoogeveen, R. W. M., Jongma, R. T. N., NoÃ«l, S., Piters, A., Schrijver, H., Schrijvers, C., Sioris, C. E., Skupin, J., Slijkhuis, S., Stammes, P., and Wuttke, M.: SCIAMACHY Level 1 data: calibration concept and in-flight calibration, Atmos. Chem. Phys., 6, 5347â€“5367, 2006. </reference>
		<reference numeration="22" content_type="text"> Liu, X., Chance, K., Sioris, C. E., and Kurosu, T. P.: Impact of using different ozone cross sections on ozone profile retrievals from Global Ozone Monitoring Experiment (GOME) ultraviolet measurements, Atmos. Chem. Phys., 7, 3571â€“3578, 2007. </reference>
		<reference numeration="23" content_type="text"> Loyola, D., Cloud retrieval for SCIAMACHY, in: Proceedings of ERS-ENVISAT Symposium, Gothenburg, Sweden, available at:  http://earth.esrin.esa.it/pub/ESA_DOC/gothenburg/282loyol.pdf, 16â€“20 October 2000. </reference>
		<reference numeration="24" content_type="text"> Loyola, D.: Automatic cloud analysis from polar-orbiting satellites using neural network and data fusion techniques, in: Proceedings of IEEE International Geoscience and Remote Sensing Symposium, 4, 2530â€“3534, 2004. </reference>
		<reference numeration="25" content_type="text"> Loyola, D. G., Coldewey-Egbers, M., Dameris, M., Garny, H., Stenke, A., Van Roozendael, M., Lerot, C., Balis, D., and Koukouli, M.: Global long-term monitoring of the ozone layer â€“a prerequisite for predictions, Int. J. Remote. Sens., accepted for publication, 2008. </reference>
		<reference numeration="26" content_type="text"> Malicet, C., Daumont, D., Charbonnier, J., Parisse, C., Chakir, A., and Brion, J.: Ozone UV spectroscopy, II: Absorption cross-sections and temperature dependence, J. Atmos. Chem., 21, 263â€“273, 1995. </reference>
		<reference numeration="27" content_type="text"> Munro, R., Eisinger, M., Anderson, C., Callies, J., Corpaccioli, E., Lang, R., Lefebvre, A., Livschitz, Y., and PÃ©rez AlbiÃ±ana, A.: GOME-2 on Metop: From in-orbit verification to routine operations, in: Proceedings of EUMETSAT Meteorological Satellite Conference, Helsinki, Finland, available at: http://www.eumetsat.int/Home/Main/Publications/index.htm, 12â€“16 June 2006. </reference>
		<reference numeration="28" content_type="text"> Paur, R. J. and Bass, A. M.: The ultraviolet cross-sections of ozone, II, Results and temperature dependence, in: Atmospheric Ozone, edited by: Zerefos, C. S., Ghazi, A., and Reidel, D., Norwell, Mass., 611â€“616, 1985. </reference>
		<reference numeration="29" content_type="text"> Platt, U.: Differential optical absorption spectroscopy (DOAS), in: Air Monitoring by Spectroscopic Techniques, edited by: Sigrist, M. W., Chemical Analysis Series, Wiley, New York, 127, 27â€“84,1994. </reference>
		<reference numeration="30" content_type="text"> Platt, U. and Stutz, J.: Differential optical absorption spectroscopy, Physics of Earth and Space Environments, doi:10.1007/978-3-540-75776-4, Springer-Verlag, Berlin Heidelberg, 2008. </reference>
		<reference numeration="31" content_type="text"> Richter, A. and Burrows, J. P.: Retrieval of Tropospheric NO2 from GOME Measurements, Adv. Space Res., 29(11), 1673â€“1683, 2002. </reference>
		<reference numeration="32" content_type="text"> Slijkhuis, S.: ENVISAT-1 SCIAMACHY Level 0 to 1c Processing Algorithm Theoretical Basis Document, ENV-ATB-DLR-SCIA-0041, Issue 4, available at: http://envisat.esa.int/services/sample_products/sciamachy/documentation/SCIAMACHY/atbd_0_to1c.pdf, 2005. </reference>
		<reference numeration="33" content_type="text"> Spurr, R. J. D.: LIDORT V2PLUS: A comprehensive radiative transfer package for UV/VIS/NIR nadir remote sensing, in: Proceedings of SPIE, 5235, Remote sensing of clouds and the atmosphere, 89â€“100, doi:10.1117/12.511103, 2004. </reference>
		<reference numeration="34" content_type="text"> Spurr, R., Loyola, D., Thomas, W., Balzer, W., Mikusch, E., Aberle, B., Slijkhuis, S., Ruppert, T., Van Roozendael, M., Lambert, J.-C., and Soebijanta, T.: GOME level 1-to-2 data processor version 3.0: a major upgrade of the GOME/ERS-2 total ozone retrieval algorithm, Appl. Opt., 44(33), 7196â€“7209, 2005. </reference>
		<reference numeration="35" content_type="text"> Van Roozendael, M., Soebijanta, V., Fayt, C., and Lambert, J.-C. (Eds.): Investigation of DOAS issues affecting the accuracy of the GDP version 3.0 total ozone product, in ERS-2 GOME GDP 3.0 implementation and delta verification, Rep. ERSE-DTEX-EOAD-TN-02_0006, 97-129, Eur. Space Res. Inst., Eur. Space Agency, Frascati, Italy, available at: http://earth.esrin.esa.it/pub/ESA_DOC/GOME/gdp3/gdp3.pdf, 2002. </reference>
		<reference numeration="36" content_type="text"> Van Roozendael, M., Loyola, D., Spurr, R., Balis, D., Lambert, J.-C., Livschitz, Y., Valks, P., Ruppert, T., Kenter, P., Fayt, C., and Zehner, C.: Ten years of GOME/ERS-2 total ozone data â€“ The new GOME data processor (GDP) version 4: 1. Algorithm description, J. Geophys. Res., 111, D14311, doi:10.1029/2005JD006375, 2006. </reference>
		<reference numeration="37" content_type="text"> Von Bargen, A., SchrÃ¶der, T., Doicu, A., Kretschel, K., Lerot, C., Van Roozendael, M., Kokhanovsky, A., Vountas, M., Bovensmann, H., Hess, M., Aberle, B., and Schreier, F.: SCIAMACHY  Level 1b-2 Data Processing: Update of Off-line Data Processor to Version 3.0, Third Workshop on the Atmospheric Chemistry Validation of ENVISAT (ACVE-3), ESA-SP-642, Frascati, 2007. </reference>
		<reference numeration="38" content_type="text"> Wang, P., Stammes, P., van der A, R., Pinardi, G., and van Roozendael, M.: FRESCO+: an improved O2 A-band cloud retrieval algorithm for tropospheric trace gas retrievals, Atmos. Chem. Phys., 8, 6565â€“6576, 2008. </reference>
	</references>
</article>

